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Nitric acid trihydrate nucleation and denitrification in the Arctic stratosphere

2014

Abstract. Nitric acid trihydrate (NAT) particles in the polar stratosphere have been shown to be responsible for vertical redistribution of reactive nitrogen (NOy). Recent observations by Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the CALIPSO satellite have been explained in terms of heterogeneous nucleation of NAT on foreign nuclei, revealing this to be an important formation pathway for the NAT particles. In state of the art global- or regional-scale models, heterogeneous NAT nucleation is currently simulated in a very coarse manner using a constant, saturation-independent nucleation rate. Here we present first simulations for the Arctic winter 2009/2010 applying a n…

Atmospheric ScienceDenitrification010504 meteorology & atmospheric sciencesForward scatterNucleationAtmospheric sciences01 natural sciences010309 opticslcsh:Chemistry0103 physical sciencesddc:550Life ScienceStratosphere0105 earth and related environmental sciencesSpectrometerozone holeChemistryAtmosphärische Spurenstoffelcsh:QC1-999Earth sciencesLidarnitric acid trihydratelcsh:QD1-99913. Climate actionPolarParticle sizelcsh:PhysicsArctic stratosphere
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